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• W2040795191 endingPage "A928" @default.
• W2040795191 startingPage "A924" @default.
• W2040795191 abstract "Neutron diffraction is a unique technique to study Li-ion batteries because of its high sensitivity toward detecting lithium ions and ability to differentiate between different cations. This information is essential for understanding the subtle structure/property relationships of active electrode materials. In this study, neutron diffraction was utilized to probe the cation disorder in LiNiO2 with and without Al3+ substitution by different synthesis processes. The powder neutron diffraction revealed that a strong oxidizer rather than Al3+-doping greatly reduces Li+ and Ni2+ mixing. The amount of Ni2+ at Li-site is 6% for Li1−x(Ni0.75Al0.25)1+xO2 synthesized from excess LiOH, while it is only 0.6% for Li1−x(Ni0.75Al0.25)1+xO2 which was synthesized from excess Li2O2. The reduction of Ni2+ at Li-sites greatly improves electrochemical performance. The substitution of Al3+ stabilizes the hexagonal lattice of Li1−xNi1+x−yAlyO2 even for highly lithium-deficient phases." @default.
• W2040795191 created "2016-06-24" @default.
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• W2040795191 date "2012-01-01" @default.
• W2040795191 modified "2023-10-18" @default.
• W2040795191 title "Probing Li-Ni Cation Disorder in Li_1−<i>x</i>Ni_{1+<i>x</i>−<i>y</i>}Al_<i>y</i>O₂Cathode Materials by Neutron Diffraction" @default.
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• W2040795191 doi "https://doi.org/10.1149/2.005207jes" @default.
• W2040795191 hasPublicationYear "2012" @default.
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