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- W2040966445 abstract "Ti films grow on Ru(0001) in a layer-by-layer mode, a (√91 × √91)R5.2 ° LEED pattern appearing at loadings close to monolayer completion. Such films are extremely active towards H2 and CO chemisorption, although in both cases no aggregation of the Ti deposit occurs as a result. The uptake of β-CO (characteristic of clean Ru) is strongly suppressed by Ti dosing: this effect is markedly nonlinear and the results suggest that islands of Ti exert a significant long-range influence on the chemisorption of CO by Ru. Isotope data show that the presence of Ti leads to the formation of dissociatively adsorbed CO, while hydrogen chemisorption results in a surface hydride species of limiting stoichiometry TiH3. This latter species decomposes at ~600 K with concomitant formation of an RuTi surface alloy; the TiH3 surface hydride is itself very active in the dissociative chemisorption of CO. The relevance of these findings to aspects of the SMSI phenomenon and to K-promoted Ru is discussed." @default.
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- W2040966445 date "1988-06-01" @default.
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- W2040966445 title "Model studies of the SMSI phenomenon I. Co and hydrogen chemistry at the Ru$z.sbnd;Ti interface" @default.
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- W2040966445 doi "https://doi.org/10.1016/0021-9517(88)90097-8" @default.
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