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- W2040972531 abstract "Plastic deformation of three amorphous polymers, such as poly(methyl methacrylate) (PMMA), poly(carbonate) (PC) and cross-linked PMMA, was investigated by low frequency Raman scattering. The induced structure modifications are found to differ in cross-linked and linear polymers. In the latter case, the deformation gives rise to a large scattering excess, maximum around 35 cm−1, which is stronger with PC than with PMMA. The intensity of this excess depends on the inclination of the shear stress direction relative to the light polarization, thus indicating a significant anisotropy in the deformed amorphous structure. In the frame of a non-continuous glassy structure model, these changes are interpreted by a partial orientation of macromolecular strands in nanometric, less cohesive zones of the matrix. In the case of a three-dimensional polymeric network, the deformation occurs through a less localized process, affecting the more cohesive regions. Similar arguments are developed for specimens that were either plastically cycled or deformed at the glass transition temperature." @default.
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- W2040972531 date "1996-03-01" @default.
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- W2040972531 title "Low frequency Raman scattering study of the nanostructure of plastically deformed polymer glasses" @default.
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- W2040972531 doi "https://doi.org/10.1016/0022-3093(95)00591-9" @default.
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