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- W2041036894 abstract "Dinuclear [Cu2(μ-OH)] fragment and its self-assembled tetranuclear part [Cu2(μ4-O)Cu2] are found in two copper(II) complexes of ligand H3bpmp: [Cu2(μ2-OH)(μ-H2bpmp)(μ1,3-NO3)][Cu2(μ2-OH)(μ-H2bpmp)(NO3)(H2O)](NO3)2·2H2O (1·2H2O) and [Cu4(μ4-O)(μ-H2bpmp)2(μ1,3-O2CCH2Ph)4] (2) [H3bpmp = 2,6-bis-[(3-hydroxy-propylimino)-methyl]-4-methylphenol]. These complexes have been synthesized and characterized by single crystal X-ray crystallography. Complex 1 showed unique reactivity with phenylacetate anions to provide 2 in which two [Cu2(μ2-OH)] units available within same crystal lattice collapsed to give [Cu4(μ4-O)] hub. Formation of the [Cu4] compound is also achieved from individual components and phenylacetate ligands, which allows an effective tuning of the self-assembly of two ligand bound [Cu2] fragments and removal of H+ from hydroxido bridges to provide oxido nucleus." @default.
- W2041036894 created "2016-06-24" @default.
- W2041036894 creator A5005489280 @default.
- W2041036894 creator A5057599116 @default.
- W2041036894 date "2013-03-01" @default.
- W2041036894 modified "2023-10-16" @default.
- W2041036894 title "New μ-hydroxido-bridged copper nitrate dimer and μ4-oxido-bridged copper phenylacetate quasi-tetrahedron: Direct synthesis and uphill conversion" @default.
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- W2041036894 doi "https://doi.org/10.1016/j.poly.2012.08.064" @default.
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