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- W2041070986 abstract "The photoreduction of 1,4-naphthoquinone in 2-propanol and 2-methyl-1-propanol at −23°C was studied with a new microsecond time resolving ESR spectrometer system. The transient alcohol radicals were identified and their relaxation times measured. The 2-propyl-2-ol radical derived from 2-propanol was found to have T1 = 1.50 μs and T2 = 1.01 μs. For the 2-methyl-1-propyl-1-ol radical derived from 2-methyl-1- propanol T1 was determined to 3.19 μs whereas T2 could not be found. The rate constants for the reaction of alcohol radicals with unexcited 1,4-naphthoquinone was measured to 6.7 × 108 ℓ s−1 mol−1 for 2-propanol and 3.2 × 108 ℓ −1 mol −1 for 2-methyl-1-propanol. The initial RPM polarisation for the alcohol radicals was measured and compared with values calculated from the microscopic theory. The calculated values were too small by a factor of two." @default.
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- W2041070986 date "1981-08-01" @default.
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- W2041070986 title "Relaxation times, rate constants, and cidep for transient alcohol radicals in the photoreduction of 1,4-naphthoquinone by microsecond time resolved ESR" @default.
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- W2041070986 doi "https://doi.org/10.1016/0301-0104(81)85178-6" @default.
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