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• W2041102316 abstract "This work reports on the nanoscale assembly of hybrid lanthanum oxide and silica structures, which form patterns of interfacial dense and porous networks. It was found that increasing the molar ratio of lanthanum nitrate to tetraethyl orthosilicate (TEOS) in an acid catalysed sol-gel process alters the expected microporous metal oxide silica structure to a predominantly mesoporous structure above a critical lanthanum concentration. This change manifests itself by the formation of a lanthanum silicate phase, which results from the reaction of lanthanum oxide nanoparticles with the silica matrix. This process converts the microporous silica into the denser silicate phase. Above a lanthanum to silica ratio of 0.15, the combination of growth and microporous silica consumption results in the formation of nanoscale hybrid lanthanum oxides, with the inter-nano-domain spacing forming mesoporous volume. As the size of these nano-domains increases with concentration, so does the mesoporous volume. The absence of lanthanum hydroxide (La(OH)3) suggests the formation of La2O3 surrounded by lanthanum silicate." @default.
• W2041102316 created "2016-06-24" @default.
• W2041102316 creator A5026237179 @default.
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• W2041102316 date "2015-02-03" @default.
• W2041102316 modified "2023-09-25" @default.
• W2041102316 title "Nanoscale assembly of lanthanum silica with dense and porous interfacial structures" @default.
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• W2041102316 doi "https://doi.org/10.1038/srep08210" @default.
• W2041102316 hasPubMedCentralId "https://www.ncbi.nlm.nih.gov/pmc/articles/4316191" @default.
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• W2041102316 hasPublicationYear "2015" @default.
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