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• W2041307052 abstract "Abstract An in situ experimental technique using radioisotopes for studying trace metal behaviour in coastal waters has been developed and results from the southern North Sea presented. Isotopes109Cd,137Cs and65Zn were adsorbed rapidly (within 25 h) by particles from the Humber and Thames estuarine plumes. The reversibility of this sorption was assessed by a series of leaching experiments and decreased in the order109Cd (removed by seawater) >65Zn (removed by 1M HCl) 137Cs (40% resistant to 1M HCl). In contrast,54Mn was deposited onto plume particles by slow oxidative precipitation which proceeded linearly. However, the protracted nature of this reaction meant that particle affinity (as quantified by a solid-solution distribution coefficient, KD) after 5 days was significantly greater than other isotopes studied; thus, 54Mn (5 × 104) >65Zn (5 × 103) >109Cd,137Cs (5 × 102). Moreover, 5-day KDs for109Cd and65Zn were enhanced by plankton compared with plume samples, whereas a137Cs association with plankton was not detectable. These trends were corroborated by KDs derived from ambient dissolved and digested particulate metal concentrations as determined by atomic absorption methods. Ambient KDs were, however, consistently an order of magnitude or more greater than their radiochemical counterparts because of an overwhelming detrital (unavailable) component of particulate metals inherent in their calculation. Accordingly, results from the radiochemical approach are favoured for incorporation into incipient shelf sea pollutant dispersal models and for assessing the potential for accumulation in the aquatic foodchain." @default.
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• W2041307052 date "1992-11-01" @default.
• W2041307052 modified "2023-09-27" @default.
• W2041307052 title "The solid-solution partitioning of trace metals in the southern North Sea—in situ radiochemical experiments" @default.
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• W2041307052 doi "https://doi.org/10.1016/0278-4343(92)90066-s" @default.
• W2041307052 hasPublicationYear "1992" @default.
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