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- W2041310050 abstract "An approach to extend the Fano–DeVoe model is presented for copolymer systems by making use of the Green’s operator method within the dipole–dipole approximation. We derive a model Hamiltonian for a system by expanding its primitive Hamiltonian in terms of a bare complete basis set consisting of zero-order one-site and two-site excitation states in the first-order perturbation theory. A generalized extension of the Fano–DeVoe theory can be given by the polarizability tensor derived for this model Hamiltonian. As a more refined way, we derive another model Hamiltonian by expanding the primitive Hamiltonian of the system in terms of the corrected complete basis set consisting of the first-order excitation states. With such model Hamiltonians, we can fabricate polarizability theories on the same footing with the exciton wave function approaches based on the usual perturbation theory. Simplified schemes for the latter model Hamiltonians are applied to the copolymer system consisting of such chromophores that ..." @default.
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- W2041310050 date "1987-08-01" @default.
- W2041310050 modified "2023-09-26" @default.
- W2041310050 title "A Linear Response Polarizability Theory for an Extended Fano–DeVoe Model with Comments on the Joint Use of Both Short- and Long-Range Inter(sub)molecular Interaction Approximations" @default.
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- W2041310050 doi "https://doi.org/10.1246/bcsj.60.2791" @default.
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