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• W2041344668 abstract "The matrix reaction of dichlorine monoxide with alkali metal atoms at high dilution in argon produces absorptions due to the appropriate alkali metal chlorides and bands near 995 and 850 cm−1 which show the calculated oxygen isotopic shift for a ClO diatomic species and are independent of the alkali metal used to generate the reaction. The 995-cm−1 feature has an appropriate chlorine isotopic counterpart for ClO. Experiments altering the concentrations of Cl2O and lithium atom reactants identify the 995-cm−1 absorption as the vibrational fundamental of ClO and the 850-cm−1 band as ClO perturbed by another molecule, perhaps the Cl2O precursor. This assignment is consistent with the conclusions of earlier matrix isolation studies of ClO species. The high Cl–O force constant in the chlorine oxide free radical is rationalized in terms of (p–p) π bonding." @default.
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• W2041344668 date "1971-10-01" @default.
• W2041344668 modified "2023-09-27" @default.
• W2041344668 title "Argon Matrix Infrared Spectrum of the ClO Radical" @default.
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• W2041344668 doi "https://doi.org/10.1063/1.1676550" @default.
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