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• W2041378032 abstract "We report the application of Mid-IR laser spectroscopy to differentiation of CO 2 sources. High-frequency isotopic CO 2 measurements (δ 13 C and δ 18 O) in urban air in Nagoya allow for the contributions of anthropogenic and biogenic CO 2 sources to be differentiated. The laser spectroscopic method, using a Mid-IR quantum cascade laser, provides us with the advantage of higher temporal resolution of the data compared to traditional isotope ratio mass spectroscopy. The relative contribution of CO 2 sources in Nagoya was found to be roughly 0.42, 0.33 and 0.25 for natural combustion, gasoline combustion and biogenic respiration in the spring, but with large short-term (hourly) variations dependent on wind direction, and long-term variations dependent on heating demand and biological seasonality. ► Mid-IR laser spectroscopy was applied for differentiation of CO 2 sources in urban air. ► High-frequency isotopic CO 2 measurements (δ 13 C and δ 18 O) were performed. ► Relative contribution of CO 2 sources showed short-term and seasonal variations. ► Relative contribution of CO 2 sources changed in different atmospheric conditions. ► A quantum cascade laser was used for the Mid-IR laser spectroscopy." @default.
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• W2041378032 date "2011-02-01" @default.
• W2041378032 modified "2023-09-24" @default.
• W2041378032 title "Observation of carbon and oxygen isotopic compositions of CO2 at an urban site in Nagoya using Mid-IR laser absorption spectroscopy" @default.
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• W2041378032 doi "https://doi.org/10.1016/j.atmosenv.2010.10.015" @default.
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