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- W2041426604 abstract "Determining the electronic coupling matrix element, V, for an electron transfer reaction is challenging both experimentally and theoretically. The magnitude of the singlet−triplet splitting (spin−spin exchange interaction), 2J, within a radical ion pair (RP) is directly related to the sum of the squares of the matrix elements that couple the RP state to the ground state and to other energetically proximate excited and ionic states. Each term in this sum is weighted by the reciprocal of the energy gap between the RP state and the particular state to which it is coupled. We present here a series of intramolecular triads with linear, rodlike structures that undergo very efficient two-step electron transfer following direct excitation of a 4-(N-piperidinyl)naphthalene-1,8-dicarboximide (6ANI) chromophore. Attachment of a p-methoxyaniline (MeOAn) donor by means of the piperazine bridge and naphthalene-1,8:4,5-bis(dicarboximide) (NI) or pyromellitimide (PI) acceptors, either directly or through a 2,5-dimethylph..." @default.
- W2041426604 created "2016-06-24" @default.
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- W2041426604 date "2003-04-18" @default.
- W2041426604 modified "2023-10-10" @default.
- W2041426604 title "Direct Measurement of Singlet−Triplet Splitting within Rodlike Photogenerated Radical Ion Pairs Using Magnetic Field Effects: Estimation of the Electronic Coupling for Charge Recombination" @default.
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- W2041426604 doi "https://doi.org/10.1021/jp0224315" @default.
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