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- W2041496636 abstract "The observed hfs coupling constant of the H2S33 molecule shows a large asymmetry although the H–S–H bond angle is known to be almost 90°. It is shown in this paper that a nonzero d character of the S–H bond orbital can explain this result. Assuming that the electron distribution is cylindrically symmetric about each S–H bond, and the radial part of the p- and d-wave functions are the same, 10.5% s character, 73.5% p character, and 16% d character is concluded for the bond orbital; 23% p character and 77 percent s character is assigned for the lone pair. If the ionic structure is neglected, the electric quadrupole moment of the S33 nucleus is estimated to be —0.11×10—24 cm2." @default.
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- W2041496636 date "1958-04-01" @default.
- W2041496636 modified "2023-09-23" @default.
- W2041496636 title "Hfs of the H2S Molecule and Its Electronic Structure" @default.
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- W2041496636 doi "https://doi.org/10.1063/1.1744215" @default.
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