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- W2041743401 abstract "Line-breadth parameters for oxygen have been determined with a Zeeman modulation spectrograph for fifteen microwave transitions occurring in the 5-mm wavelength region. Measured values lie in the range 0.0319 to 0.0516 ${mathrm{cm}}^{ensuremath{-}1}$/atmos, with a population weighted mean of 0.0475 ${mathrm{cm}}^{ensuremath{-}1}$/atmos. Investigation of the variation of the line-breadth parameter as a function of $K$, the rotational angular momentum quantum number, reveals greater line-breadth for the most populated states. This leads to an interpretation of the self-broadening collision process as a mechanism involving not only the quadrupole-quadrupole and polarizability interactions predicted theoretically, but also a rotational resonance interaction.Measurements are also reported for the line-breadths of oxygen transitions broadened by the perturbing molecules ammonia, nitrous oxide, nitrogen, and argon. Collision diameters are then determined for these molecules, and the results are shown to compare favorably with results from kinetic theory and from ammonia-broadening experiments. Interpretations of these data also strengthen the rotational resonance interpretation. A line-breadth parameter is calculated for air." @default.
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- W2041743401 date "1952-08-15" @default.
- W2041743401 modified "2023-09-25" @default.
- W2041743401 title "Line-Breadths of the Microwave Spectrum of Oxygen" @default.
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- W2041743401 doi "https://doi.org/10.1103/physrev.87.561" @default.
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