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• W2041771687 abstract "We scrutinized the reaction mechanism of CO2 methanation catalyzed by a Pd-MgO/SiO2 catalyst. Density functional theory studies showed that MgO and Pd nanoparticles play completely different roles. We found that MgO initiates the reaction by binding a CO2 molecule, forming a magnesium carbonate species on the surface, and that a supply of atomic H is essential for further hydrogenation of magnesium carbonate to methane. A CO2temperature-programmed desorption study gives credence to our findings on the role of MgO. Our results confirm the bifunctional mechanism of CO2 methanation by a Pd-MgO/SiO2 catalyst." @default.
• W2041771687 created "2016-06-24" @default.
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• W2041771687 date "2010-03-26" @default.
• W2041771687 modified "2023-10-11" @default.
• W2041771687 title "Bifunctional Mechanism of CO₂ Methanation on Pd-MgO/SiO₂ Catalyst: Independent Roles of MgO and Pd on CO₂ Methanation" @default.
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• W2041771687 doi "https://doi.org/10.1021/jp100938v" @default.
• W2041771687 hasPublicationYear "2010" @default.
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