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• W2042499100 abstract "We study the trajectories of a single colloidal particle as it hops between two energy wells which are sculpted using optical traps. Whereas the dynamical behaviors of such systems are often treated by master-equation methods that focus on particles as actors, we analyze them instead using a trajectory-based variational method called maximum caliber (MaxCal). We show that the MaxCal strategy accurately predicts the full dynamics that we observe in the experiments: From the observed averages, it predicts second and third moments and covariances, with no free parameters. The covariances are the dynamical equivalents of Maxwell-like equilibrium reciprocal relations and Onsager-like dynamical relations." @default.
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• W2042499100 date "2009-07-31" @default.
• W2042499100 modified "2023-10-16" @default.
• W2042499100 title "Trajectory Approach to Two-State Kinetics of Single Particles on Sculpted Energy Landscapes" @default.
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• W2042499100 doi "https://doi.org/10.1103/physrevlett.103.050603" @default.
• W2042499100 hasPubMedCentralId "https://www.ncbi.nlm.nih.gov/pmc/articles/3273425" @default.
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