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• W2042553571 abstract "The present work aims to quantitatively measure HCN in a low pressure premixed CH4/N2O/O2/N2 flame after gas probe sampling. For that purpose, the (0 0 3)–(0 0 0) band of HCN has been selected for the first time for HCN monitoring. This band was chosen because it lies in a wavelength range (1.036 μm) easily reachable by commercial dye laser combined with Raman cell shifter. The line strengths of its main R branches are 30 times lower than the transitions lying at 1.5 μm generally used. The sensitivity was achieved using pulsed CRDS technique in a long absorption cell (1 m). The required wavelength is generated from the first stokes radiation of hydrogen after 724 nm pumping. First, absorption spectra of HCN diluted in N2 have been obtained and compared to simulated spectra of the R-branch. The very good agreement between the experimental and simulated spectra, both in line position and absolute intensity, allows to validate our strategy and the experimental setup. Second the HCN profile in the flame was determined by measuring the integrated spectral absorptivity around the R(7) transition line of HCN. The profile of the HCN mole fraction along the flame has been measured with a peak value equal to 600 ppm. The technique implemented allows detecting HCN in the limit of 2.5 × 1013 molecule cm−3 with an accuracy of 20%." @default.
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• W2042553571 date "2013-01-01" @default.
• W2042553571 modified "2023-10-17" @default.
• W2042553571 title "HCN quantitative measurement in a laminar low pressure flame at 1036 nm using pulsed CRDS technique" @default.
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• W2042553571 doi "https://doi.org/10.1016/j.proci.2012.06.067" @default.
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