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• W2042783251 abstract "The study of chiral adsorbed molecules is important for an analysis of enantioselectivity in heterogeneous catalysis. Here we show that such molecules can be identified through circular dichroism in core-level photoemission arising from the chiral carbon atoms in stereoisomers of 2,3-butanediol molecules adsorbed on Si(100), using circularly polarized x rays. The asymmetry in the carbon 1s intensity excited by right and left circularly polarized light is readily observed, and changes sign with the helicity of the radiation or handedness of the enantiomers; it is absent in the achiral form of the molecule. This observation demonstrates the possibility of determining molecular chirality in the adsorbed phase." @default.
• W2042783251 created "2016-06-24" @default.
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• W2042783251 date "2005-09-02" @default.
• W2042783251 modified "2023-10-18" @default.
• W2042783251 title "Atom-Specific Identification of Adsorbed Chiral Molecules by Photoemission" @default.
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• W2042783251 doi "https://doi.org/10.1103/physrevlett.95.107601" @default.
• W2042783251 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/16196965" @default.
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