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- W2042882015 abstract "Desorption of NO molecules from Pd(110) at 490 K mediates the emission of N2 and N2O. The N2 emitted at 490 K has a spatial distribution with a maximum intensity at 38° from the surface normal in the [001] direction, which is expressed by 0.9 cos4.2 θ + 1.9 cos46(θ ± 38°). In contrast, the desorptions of NO and N2O at 490 K follow a cos θ and a cos2θ distribution, respectively. Desorption of 14NO from a 15N preadsorbed Pd(110) surface mediated predominant desorption of 14N15N in the off-normal distribution, whereas the 15N2 desorption by the recombination of 15N atoms follows a cos6θ−cos7θ distribution. These results suggest that the reaction coordinate for the N(ad) + NO(ad) → N2↑ + O(ad) reaction is responsible for the off-normal emission of N2. On the other hand, N2 produced by a catalytic reaction of NO + H2 at 600 K follows a cos θ distribution. On the basis of these experiments, we believe that the spatial distributions of desorbing molecules for this system are related to the reaction mechanism, especially, the orientation of the coordinate for the desorption process." @default.
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- W2042882015 title "Mechanism for the Off-Normal Emission of N<sub>2</sub> in the Desorption-Mediated Reaction of NO on a Pd(110) Surface" @default.
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- W2042882015 doi "https://doi.org/10.1021/jp9903918" @default.
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