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- W2042923631 abstract "An optically pumped system of rubidium has been used as a probe to measure the concentration of free radicals present during the vacuum-ultraviolet photolysis of five hydrocarbons. The mechanism for this measurement is the reduction of the relaxation time of the oriented rubidium in the presence of radicals, due to the large spin exchange interaction between the two species. Measurements were made at two different pressures each on methane, ethane, propane, butane, and isobutane; from this both relative and absolute approximate quantum yields for radical production are determined. Separate detection of hydrogen atoms during the photolysis, through spin exchange coupled electron spin resonance, was reported briefly in an earlier note and is discussed more fully here. This method of directly detecting free-radical intermediates appears to be a useful complement to standard experiments in which reaction mechanisms are deduced from analysis of final products of the photolysis." @default.
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- W2042923631 date "1967-08-15" @default.
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- W2042923631 title "Use of Optical Pumping to Detect Free Radicals during a Gas‐Phase Photolysis" @default.
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- W2042923631 doi "https://doi.org/10.1063/1.1712088" @default.
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