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• W2043291504 abstract "A natural smectite clay (STx-1, USA) was ion-exchanged with Al, Fe or pillared with polyoxocations of the same metals. Samples were also prepared by combining these two treatments. The prepared solids were characterized by X-ray fluorescence (XRF), X-ray diffraction (XRD), thermogravimetric analysis (TGA), TPD of ammonia and N2 adsorption. The catalytic activity was evaluated by using the isomerization of 1-butene at 300 °C. XRF results showed an increase in the content of Al or Fe thus giving evidence that these metals were effectively exchanged or deposited over the starting material. Al- and Fe-pillared clays showed a significant increase of the surface area. Ion-exchanged clays showed similar surface areas to that of the starting clay. From XRD patterns only the Al-pillared clay gave an increase of the d-spacing. The synthesized pillared clays were superior catalysts for the isomerization of 1-butene than the ion-exchanged clays; the ion-exchanged/pillared clays showed a similar catalytic behavior as that of the parent pillared clays. The Al-pillared clay was the best catalyst for the reaction and its efficiency was related to the high acidity and high surface area." @default.
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• W2043291504 date "2008-01-01" @default.
• W2043291504 modified "2023-10-16" @default.
• W2043291504 title "Isomerization of 1-butene catalyzed by ion-exchanged, pillared and ion-exchanged/pillared clays" @default.
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• W2043291504 doi "https://doi.org/10.1016/j.apcata.2007.09.043" @default.
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