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- W2043892885 abstract "The role of the potential of intermolecular force in determining properties of gases at elevated temperatures is discussed, and the following points are emphasized. (a) The calculation of accurate values of such properties requires potential parameters which are valid at interaction distances which are important at the temperatures in question. (b) Extrapolation of potentials obtained from low temperature properties for calculation of high temperature properties is, in general, not justified, and leads to values of transport coefficients and second virial coefficients which differ considerably from those calculated from potentials based on the elastic scattering of high energy molecular beams. (c) The high temperature range, in which such beam potentials are useful, is not determined by the kinetic energy of the beam particles, but by the small fraction of this energy which is converted into potential energy in the scattering process. For purposes of illustration, coefficients of viscosity and self-diffusion, isotopic reduced thermal diffusion ratios, and second virial coefficients for helium, argon and nitrogen at 1000°, 5000° and 15000° K have been calculated from extrapolated potentials, Lennard-Jones (12-6) and modified Buckingham (exp-6), and from beam potentials." @default.
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- W2043892885 date "1958-12-01" @default.
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- W2043892885 title "On the calculation of properties of gases at elevated temperatures" @default.
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- W2043892885 doi "https://doi.org/10.1016/0010-2180(58)90033-6" @default.
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