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- W2043952125 abstract "A theory of time-resolved photoelectron spectroscopy from coherent rotational wavepackets is developed within a density matrix framework, expressing the signal as a partial wave series of rotational operators that tie the underlying electronic and rotational dynamics. The theory is applied to suggest and explore two potential applications of time- and angle-resolved photoelectron signals. First, we consider the possibility of extracting the bound-free electronic dipole matrix elements that underlie the ionization process from experimental data. Next, we investigate the extent to which photoelectron images could serve to map the time-evolving rotational probability distribution, thus providing insights into rotational coherences." @default.
- W2043952125 created "2016-06-24" @default.
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- W2043952125 date "2012-09-24" @default.
- W2043952125 modified "2023-09-26" @default.
- W2043952125 title "On the information content of time- and angle-resolved photoelectron spectroscopy" @default.
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- W2043952125 doi "https://doi.org/10.1088/0953-4075/45/19/194012" @default.
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