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• W2043956558 abstract "Using the acetic acid/Si(001) system as an illustrative example, we discuss the limits and opportunities of ``chemical analogy'' as a paradigm to rationalize chemisorption processes on surfaces. Recent proposals that acetic acid chemisorption results in a bidentate, single-dehydrogenated product are based on earlier findings for the acetic acid/Ge(001) system. In contrast, the well-characterized reaction of acetone with Si(001) suggests that acetic acid chemisorption leads to the loss of two hydrogen atoms from the molecule. Density-functional calculations resolve this ambiguity, finding the latter structure model to be thermodynamically preferred and kinetically viable." @default.
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• W2043956558 date "2011-10-04" @default.
• W2043956558 modified "2023-09-27" @default.
• W2043956558 title "Acetic acid on silicon (001): An exercise in chemical analogy" @default.
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• W2043956558 doi "https://doi.org/10.1103/physrevb.84.153302" @default.
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