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• W2043970965 startingPage "1550" @default.
• W2043970965 abstract "The relative partial molar enthalpies, Δ H̄ SiO2 , of SiO 2 in SiO 2 –M 2 O (M = Li, Na, K and Cs) binary and SiO 2 –CaO–Al 2 O 3 ternary melts were directly measured by drop‐solution calorimetry at 1465 K and 1663 K. Δ H̄ SiO2 changes from exothermic to endothermic as silica content increases, confirming the tendency toward immisciblity seen from activity measurements. It is concluded that Δ H̄ SiO2 is negative due to acid‐base reactions and charge‐coupled substitutions when the melt is composed of fewer Q 4 and more Q 3 and Q 2 species, but positive due to structural strain when the melt is composed of mostly Q 4 species. The Δ H̄ SiO2 obtained by calorimetry is a useful measure of basicity, when comparing different alkali and alkaline earth oxides." @default.
• W2043970965 created "2016-06-24" @default.
• W2043970965 creator A5000443794 @default.
• W2043970965 creator A5022913608 @default.
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• W2043970965 date "2004-08-01" @default.
• W2043970965 modified "2023-10-07" @default.
• W2043970965 title "Direct Measurement of Relative Partial Molar Enthalpy of SiO₂in SiO₂-M₂O (M=Li, Na, K, Cs) Binary and SiO₂-CaO-Al₂O₃Ternary Melts" @default.
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• W2043970965 doi "https://doi.org/10.1111/j.1551-2916.2004.01550.x" @default.
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