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• W2043975981 abstract "We discuss the reactive sputter deposition of metal oxide nanolaminates on unheated substrates using four archetypical examples: ZrO2–Al2O3, HfO2–Al2O3, ZrO2–Y2O3, and ZrO2–TiO2. The pseudobinary bulk phase diagrams corresponding to these nanolaminates represent three types of interfaces. I. Complete immiscibility (ZrO2–Al2O3 and HfO2–Al2O3). II. Complete miscibility (ZrO2–Y2O3). III. Limited miscibility without a common end-member lattice (ZrO2–TiO2). We found that, although reactive sputter deposition is a far-from-equilibrium process, thermodynamic considerations strongly influence both phase formation within layers and at interfaces. We show that pseudobinary phase diagrams can be used to predict interfacial cation mixing in the nanolaminates. However, size effects must be considered to predict specific structures. In the absence of pseudoepitaxy, size effects play a significant role in determining the nanocrystalline phases that form within a layer (e.g. tetragonal ZrO2, tetragonal HfO2, and orthorhombic HfO2) and at interfaces (e.g. monoclinic (Zr,Ti)O2). These phases are not bulk standard temperature and pressure phases. Their formation is understood in terms of self-assembly into the lowest energy structure in individual critical nuclei." @default.
• W2043975981 created "2016-06-24" @default.
• W2043975981 creator A5020436041 @default.
• W2043975981 date "2008-06-09" @default.
• W2043975981 modified "2023-10-01" @default.
• W2043975981 title "Reactive sputter deposition of metal oxide nanolaminates" @default.
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• W2043975981 doi "https://doi.org/10.1088/0953-8984/20/26/264006" @default.
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