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• W2044309223 abstract "A dynamical semigroup Fokker–Planck equation, which meanwhile satisfies also the semiclassical detailed-balance relation at arbitrary temperatures, is constructed and further applied to nonlinear spectroscopic processes of two-surface molecular systems in condensed phases. Included in dissipation are the T1-vibrational relaxation and the pure T2-dephasing in both nuclear and electronic degrees of freedom. A mixed Heisenberg–Schrödinger picture of the field-dressed optical response function is proposed to efficient evaluation of pulsed-laser spectroscopies. Numerical simulations are carried out in a model one-dimensional dissipative Morse molecular system. Both the pump–probe absorption and the time-frequency resolved fluorescence spectra are demonstrated and analyzed in detail in terms of the underlying dissipative dynamics." @default.
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• W2044309223 date "2001-03-01" @default.
• W2044309223 modified "2023-10-01" @default.
• W2044309223 title "Dynamical semigroup Fokker–Planck equation approach to transient absorption and fluorescence upconversion spectroscopies" @default.
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• W2044309223 doi "https://doi.org/10.1063/1.1344608" @default.
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