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- W2044509911 abstract "Using the AVCC-1OS (azimuthal and vibrational close-coupled, infinite-order sudden) method, we have calculated efficiencies for vibrational relaxation of glyoxal in collisions with He and Ar at room temperature. For glyoxal-d2 (deuterated glyoxal) + He the calculated efficiency P( 0°, k = 0→71) is in reasonable agreement with experiment, but for glyoxal-d2 + Ar the calculated v of P(0°, k=0→71) is much lower than the experimental value. While part of the discrepancy may be due to the sudden approximation (to the sl nevertheless suggest that, especially for heavier collision partners, the experimental values of P(0°→71) should be much too high because the question of how rotational relaxation should affect the measurement of vibrationally relaxed and unrelaxed emission was not considered in the experiment. For glyoxal-d2 + He, the calculated efficiencies P(81→61) and P(81→8171) agreement with experiment. Because the frequency difference between the ν6 and the ν8 modes is much smaller in glyoxal-h2 (“normal” or protonated glyoxal), for glyoxal-h2 + He the calculated efficiency P(81→61) is much higher than for glyoxal-d2 + He." @default.
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- W2044509911 date "1991-10-01" @default.
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- W2044509911 title "Vibrational relaxation of glyoxal in collisions with He and Ar" @default.
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- W2044509911 doi "https://doi.org/10.1016/0301-0104(91)80096-z" @default.
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