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- W2044549019 abstract "SAPO-11 exhibited a high caprolactam yield for the vapour phase Beckmann rearrangement of cyclohexanone oxime to caprolactam. At 663 K, the oxime conversion is 99,9% with a caprolactam selectivity around 85.7%. The effect of silicon content of the SAPO-11 on the catalytic efficiency is compared with aluminosilicate having MFI structure. SAPO-11 is the best catalyst for the reaction among the investigated catalysts, ALPO4-11 on silica carrier, silynated zeolite and silynated SAPO-11. Acid sites with medium strength (Si/Al > 10 000) are very active in the rearrangement reaction." @default.
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- W2044549019 date "1996-03-01" @default.
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- W2044549019 title "Vapour phase beckmann rearrangement of cyclohexanone oxime over SAPO-11 molecular sieve" @default.
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- W2044549019 doi "https://doi.org/10.1016/0926-860x(95)00303-7" @default.
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