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- W2044549148 abstract "We have used a white light continuum generated with ultrashort laser pulses from a Ti:sapphire laser system as the radiation source for second-harmonic generation measurements. The white light continuum provides easily tuned radiation for experiments requiring a range of wavelengths. Despite the small coherence length of the radiation, parametric processes, such as second-harmonic generation, are possible with this source. In particular, surface second-harmonic generation using the white light continuum is reasonable because the extent of the interface is much smaller than the coherence length of the radiation. We demonstrate second-harmonic generation from a gold surface and show that surface second-harmonic generation using the white light continuum can be used to measure absorption spectroscopy of molecules adsorbed to surfaces via resonance enhancement of the surface second-harmonic signals." @default.
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- W2044549148 date "1997-09-01" @default.
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- W2044549148 title "White light continuum as a tunable radiation source for second-harmonic generation experiments" @default.
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- W2044549148 doi "https://doi.org/10.1063/1.1148290" @default.
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