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• W2044612835 abstract "Specific bond breaking reactions are observed on surface defects on Fe(llO) when adsorbed layers of CCl4 or CCl2F2 are heated. For CCl2F2, CF bonds are broken at defect sites, producing FeF2 species and the: CCl2 diradical. For CC14, FeCl2species a : CCl2 species are produced at defect sites. It is shown that the yield of both: CCl2 and the corresponding iron dihalide may be enhanced by using Ar+ bombardment to produce surface defects (in a controlled manner) prior to halocarbon adsorption and reaction. Evidence for iron dihalide surface migration to produce clusters on defect sites is presented. Annealing experiments show that defects produced by Ar+ bombardment may be annealed away at temperatures below 400 K, while the defects which are naturally present on the crystal cannot be removed by annealing to T #62; 800 K." @default.
• W2044612835 created "2016-06-24" @default.
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• W2044612835 date "1990-06-01" @default.
• W2044612835 modified "2023-09-27" @default.
• W2044612835 title "The role of surface defects in chemisorptive molecular dissociation — Enhancement of halocarbon reactions on Fe(110)" @default.
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• W2044612835 doi "https://doi.org/10.1016/0039-6028(90)90591-u" @default.
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