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• W2044720618 abstract "In this study, we apply a self-consistent field theory of polymers to study the structures of a symmetric diblock copolymer in parallel substrates filled with square-pillar arrays in which the substrates and pillars exhibit a weak preference for one block of the copolymer. Three classes of structures, i.e., lamellae, perpendicular cylinders, and bicontinuous structures, are achieved by varying the polymer film thickness, the pillar pitch (the distance between two centers of the nearest neighboring pillars), the gap and rotation of the pillars. Because of the confinement along horizontal directions imposed by the pillar array, eight novel types of perpendicular lamellar structures and eight novel types of cylindrical structures with various shapes and distributions occur. In the hybridization states of the parallel and perpendicular lamellar structures, several novel bicontinuous structures such as the double-cylinder network, pseudo-lamellae, and perforated lamellar structure are also found. By comparing the free energies of the various possible structures, the antisymmetric parallel lamellae are observed to be stable with the larger pillar gap at a certain film thickness. The structural transformations between the alternating cylindrical structures (alternating cross-shaped, square-shaped, and octagonal perpendicular cylinders) and parallel lamellae with increasing film thickness or pillar gap are well explained by the modified strong separation theory. Our results indicate that array confinement can be an effective method to prepare novel polymeric nanopattern structures." @default.
• W2044720618 created "2016-06-24" @default.
• W2044720618 creator A5062839628 @default.
• W2044720618 creator A5072810565 @default.
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• W2044720618 date "2012-02-17" @default.
• W2044720618 modified "2023-09-26" @default.
• W2044720618 title "Phase segregation of a symmetric diblock copolymer in constrained space with a square-pillar array" @default.
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• W2044720618 doi "https://doi.org/10.1063/1.3685220" @default.
• W2044720618 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/22360259" @default.
• W2044720618 hasPublicationYear "2012" @default.
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