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- W2044737163 abstract "A discussion is presented of the relation between the film thickness d and the coexisting vapor pressure P for a physisorbed film. The theory of Dzyaloshinskii, Lifshitz, and Pitaevskii (DLP) is used to calculate the chemical potential ensuremath{Delta}ensuremath{mu}ensuremath{equiv}-ensuremath{gamma}(d)${d}^{mathrm{ensuremath{-}}3}$ relative to the value for bulk liquid. The relation is established between the DLP theory and a many-body expansion, of which the Frenkel-Halsey-Hill (FHH) theory is a first approximation to the nonretarded limit. Numerical calculations are performed for the cases of $^{4}mathrm{He}$, Ne, ${mathrm{H}}_{2}$, ${mathrm{N}}_{2}$, Ar, ${mathrm{O}}_{2}$, ${mathrm{CH}}_{4}$, Kr, and Xe films on glass, gold, graphite, Si, quartz, and Al. Typically, the effect of retardation is to reduce the thickness by 20% for densuremath{sim}200 Ar{}. The function ensuremath{gamma}(d) is shown to have a universal retardation behavior with a thickness scale (${d}_{1/2}$) depending on both adsorbate and substrate characteristic frequencies." @default.
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- W2044737163 date "1988-07-15" @default.
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- W2044737163 title "Retardation and many-body effects in multilayer-film adsorption" @default.
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- W2044737163 doi "https://doi.org/10.1103/physrevb.38.987" @default.
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