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- W2044772498 abstract "Abstract The results of the search for the A → X radiative relaxation of haloethylene cations in the gaseous phase are reported. Only in the case of cis-1,2-difloroethylene cation was an emission spectrum detected. It is identified as the A 2 A 1 → X 2 B 1 band system on the basis of photoelectron spectroscopic measurements. An assignment of the emission bands yields the vibrational frequencies of four of the A 1 fundamentals (under C 2 , symmetry) for the X state and one for the A state. Well resolved Ne(I) photoelectron spectra of cis- and trans-1,2-difluoroethylene are presented, from which some vibrational frequencies for these cations in the X and A states are also obtained. The lifetimes of cis-1,2-difluoroethylene cation in the lowest vibrational levels of the A 2 A 1 state have been measured. The decay of this cation is unusual as these levels are depleted both by, radiative, and pathways leading to fragment ions (C 2 HF + ). The lack of detectable emissions with other fluoro-, chloro- and bromo-ethylene cations is discussed and the likely symmetries of the A states are proposed." @default.
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- W2044772498 date "1979-11-01" @default.
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- W2044772498 title "à 2A1 → X̃ 2B1 emission spectrum of cis-1,2-difluoroethylene cation and the non-radiation decay of the à states of the haloethylene cations in the gaseous phase" @default.
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- W2044772498 doi "https://doi.org/10.1016/0301-0104(79)80069-5" @default.
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