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• W2044794223 endingPage "277" @default.
• W2044794223 startingPage "271" @default.
• W2044794223 abstract "Green hydrogen is identified as one of the prime clean energy carriers due to its high energy density and a zero emission of CO2. A possible solution for the transport of H2 in a safe and low-cost way is in the form of liquid organic hydrogen carriers (LOHCs). As an alternative to loading LOHC with H2 via a two-step procedure involving preliminary electrolytic production of H2 and subsequent chemical hydrogenation of the LOHC, we explore here the possibility of electrochemical hydrogen storage (EHS) via conversion of proton of a proton donor into a hydrogen atom involved in covalent bonds with the LOHC (R) via a proton-coupled electron transfer (PCET) reaction: 2nH++2ne-+Rox↔nH20Rred. We chose 9-fluorenone/fluorenol (Fnone/Fnol) conversion as such a model PCET reaction. The electrochemical activation of Fnone via two sequential electron transfers was monitored with in-situ and operando spectroscopies in absence and in presence of different alcohols as proton donors of different reactivity, which enabled us to both quantify and get the mechanistic insight on PCET. The possibility of hydrogen extraction from the loaded carrier molecule was illustrated by chemical activation." @default.
• W2044794223 created "2016-06-24" @default.
• W2044794223 creator A5031655715 @default.
• W2044794223 creator A5040063830 @default.
• W2044794223 date "1985-08-01" @default.
• W2044794223 modified "2023-09-26" @default.
• W2044794223 title "Solvent effects on the redox potentials of benzoquinone" @default.
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• W2044794223 doi "https://doi.org/10.1016/0022-0728(85)80094-2" @default.
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