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• W2044974589 abstract "The inner-shell photoionization of unoriented camphor molecules by circularly polarized light has been investigated from threshold to a photoelectron kinetic energy of ∼65 eV. Photoelectron spectra of the carbonyl C 1s orbital, recorded at the magic angle of 54.7° with respect to the light propagation direction, show an asymmetry of up to 6% on change of either the photon helicity or molecular enantiomer. These observations reveal a circular dichroism in the angle resolved emission with an asymmetry between forward and backward scattering (i.e., 0° and 180° to the light beam) which can exceed 12%. Since the initial state is an atomiclike spherically symmetric orbital, this strongly suggests that the asymmetry is caused by final-state effects dependent on the chiral geometry of the molecule. These findings are confirmed by electron multiple scattering calculations of the photoionization dynamics in the electric-dipole approximation." @default.
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• W2044974589 date "2004-03-01" @default.
• W2044974589 modified "2023-10-13" @default.
• W2044974589 title "Photoelectron circular dichroism in core level ionization of randomly oriented pure enantiomers of the chiral molecule camphor" @default.
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• W2044974589 doi "https://doi.org/10.1063/1.1651474" @default.
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