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• W2045124633 startingPage "4427" @default.
• W2045124633 abstract "Rovibrational FTIR spectra of Ni(CO)4 and Fe(CO)5 have been recorded in supersonic argon expansions at resolutions up to 0.004 cm−1. Rotational temperatures as low as 4 K for the ν6 band of Fe(CO)5 and 6 K for the ν5 band of Ni(CO)4 have been determined from the populations of the rotational levels, and an efficient vibrational cooling has been evidenced by the large reduction of hot band absorptions. An analytical model including the instrumental line shapes and the intensity distribution is proposed to enable simulations of overlapping rovibrational transitions of symmetric top molecules. The spectroscopic study of the ν6 and ν10 stretching bands of Fe(CO)5 yielded the following parameters (3σ uncertainties in parenthesis): ν0=2038.106 97(91) cm−1, B6=0.026 797(12) cm−1, and B0=0.026 826(10) cm−1 for the 610 transition, ν0=2015.5513(12) cm−1, ΔA10=−0.000 086(5) cm−1, B10=0.026 786(4) cm−1, and ξ10=−0.049(3) for the 1010 transition based on the literature value of A0." @default.
• W2045124633 created "2016-06-24" @default.
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• W2045124633 date "1996-03-22" @default.
• W2045124633 modified "2023-10-03" @default.
• W2045124633 title "High resolution Fourier transform infrared spectroscopy of the ν6 and ν10 bands of jet-cooled Fe(CO)5" @default.
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• W2045124633 doi "https://doi.org/10.1063/1.471195" @default.
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