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• W2045175500 startingPage "73" @default.
• W2045175500 abstract "Absorption and stimulated emission of microwaves has been observed in the 3 cm MODR spectrum of the photo-excited triplet state of symmetric tetrachlorobenzene (s-TCB) in a durene host crystal at liquid helium temperatures. Studies of the relative intensities of the “Δms + ± 1” transitions as a function of temperature, with the magnetic field directed along molecular fine structure axes, have been used to determine the absolute signs of the zero-field (ZF) parameters. Combining these results with those from experiments done in zero field, it is found that D = +0.1518 and E = +0.02908 cm−1. The signs of the ZF parameters in the π,π‡ triplet states of aromatic molecules are discussed, and it is shown that the sign of E in s-TCB and other substituted benzenes such as p-dichlorobenzene can be predicted using simple molecular orbital considerations." @default.
• W2045175500 created "2016-06-24" @default.
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• W2045175500 date "1972-07-01" @default.
• W2045175500 modified "2023-10-16" @default.
• W2045175500 title "The absolute signs of the zero-field parameters from microwave-optical double resonance (MODR) spectroscopy: 1,2,4,5-tetrachlorobenzene in durene" @default.
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• W2045175500 doi "https://doi.org/10.1016/0009-2614(72)87019-2" @default.
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