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- W2045227457 abstract "We report a new host molecule in which one diethylene glycol chain (i.e., a loop possessing only three oxygen atoms) incorporated along with two phenolic aromatic rings is linked by a xylene spacer into a macroring. The design of the molecular structure of this macrocycle amplifies any potential [cation...pi], [N+-H...pi], and [N+C-H...pi] interactions between the dibenzylammonium (DBA+) ion and the phenolic rings of the macrocycle; as such, these species display a very strong binding affinity in CD3NO2 (Ka = 15,000 M(-1)). The macroring also coordinates to bipyridinium ions in a [2]pseudorotaxane fashion, which makes it the smallest macrocycle (i.e., a 25-membered ring) known to complex both DBA+ and bipyridinium ions in solution. To confirm unambiguously that these pseudorotaxanes exist in solution, we synthesized their corresponding interlocked molecules, namely rotaxanes and catenanes." @default.
- W2045227457 created "2016-06-24" @default.
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- W2045227457 date "2006-02-11" @default.
- W2045227457 modified "2023-09-30" @default.
- W2045227457 title "Is [N<sup>+</sup>−H···O] Hydrogen Bonding the Most Important Noncovalent Interaction in Macrocycle−Dibenzylammonium Ion Complexes?" @default.
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- W2045227457 doi "https://doi.org/10.1021/jo052411+" @default.
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