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- W2045242826 abstract "Abstract Unimolecular fragmentation and bimolecular reactions with HCl of water clusters which nominally contain Mg + cations were studied in an FT-ICR spectrometer. A cluster fragmentation and successive evaporation of single water molecules occurring on a millisecond timescale and driven by ambient black body radiation is triggering interesting intracluster reactions. Below a certain critical size (∼17 water molecules) MgOH + forms, and a hydrogen atom is ejected. Similarly bimolecular reactions of Mg aq + clusters with HCl result in a release of H atom and formation of MgCl aq + . Both findings can be rationalized by assuming that the solvated Mg + cations actually detach an additional electron forming a Mg aq 2+ and e aq − within clusters with more than 17 water molecules. Mg + formed by recombination when not enough solvent is available to stabilize the separate charged species then reacts with a water molecule resulting in H-atom formation. Detailed studies of the ion reactions and fragmentation provide additional insights into the structure and stability of solvated magnesium cations." @default.
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- W2045242826 date "1998-12-01" @default.
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- W2045242826 title "Stability and reactivity of hydrated magnesium cations" @default.
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- W2045242826 doi "https://doi.org/10.1016/s0301-0104(98)00278-x" @default.
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