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- W2045254767 abstract "This work concerns amorphous poly(ethylene oxide) (PEO) rubbery electrolytes with new lithium salts, LiN(CF3CO)2 and Li[CF3SO2N(CH2)3OCH3] (LiMPSA), which contain carbonyl or ether groups in their anions. Although these salts are markedly less conductive than LiN(CF3SO2)2 or LiClO4, one of them (LiMPSA) yields a large fraction of a species that promotes lithium transport through back diffusion under polarization in Li/PEO–LiX/Li symmetrical cells. Polarization experiments carried out on similar cells filled with PEO–LiX–KX, mixed-alkali electrolytes show that this species is a LiX−2 complex of lower mobility than Li+ in PEO. In turn, these experiments reveal that LiN(CF3CO)2 yields a large fraction of LiX ion pairs more mobile than Li+ in PEO. These features, which are founded on theoretical models for polarization of PEO–LiX–KX electrolytes between lithium electrodes, agree with other properties (Tg elevation and conductivity) of the present systems." @default.
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- W2045254767 date "1998-04-01" @default.
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- W2045254767 title "Evidence for ion pairs and/or triple ions from transport measurements in mixed-alkali polyether electrolytes" @default.
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- W2045254767 doi "https://doi.org/10.1016/s0013-4686(97)10076-7" @default.
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