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- W2045259223 abstract "Pressurized-water-reactor spent fuel from oxidation tests at 420 to 450 K in air was examined by transmission electron microscopy to determine the mechanism of initial oxidation beyond UO2. At oxygen/metal ratios to 2.13, the fuel oxidized internally by forming U4O9 along grain boundaries and by advancing coherent U4O9/UO2 interfaces into the UO2 grains. Grain boundary cracking accompanied U4O9 formation. The U4O9 in irradiated fuel lacked long-range order, but was readily identified by the presence of diffuse extra reflections in electron diffraction. The tendency of spent fuel to internal oxidation is attributed to rapid penetration of oxygen along grain boundaries coated with closely spaced fission gas microbubbles." @default.
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- W2045259223 date "1989-08-01" @default.
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- W2045259223 title "Microstructural examination of oxidized spent PWR fuel by transmission electron microscopy" @default.
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- W2045259223 doi "https://doi.org/10.1016/0022-3115(89)90221-3" @default.
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