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• W2045320997 abstract "We use the technique of electro-magnetically induced transparency (EIT) to probe the effect of attractive dipole-dipole interactions in a highly excited Rydberg gas. The transient character of the EIT response is investigated by rapidly scanning the probe laser through resonance. We characterize the resulting cooperative optical non-linearity as a function of probe strength, density and scan direction. For the 58D$_{5/2}$ Rydberg state, an atom density of $1.6times10^{10} $cm$^{-3}$ and a positive frequency scan we measure a third-order non-linearity of $chi^{(3)}=5times 10^{-7}$ m$^2$V$^{-2}$. For the reverse scan we observe a second order non-linearity of $chi^{(2)}=5times 10^{-6}$ mV$^{-1}$. The contrasting behaviour can be explained in terms of motional effects and resonant excitation of Rydberg pairs." @default.
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• W2045320997 date "2011-09-14" @default.
• W2045320997 modified "2023-09-27" @default.
• W2045320997 title "Optical non-linearity in a dynamical Rydberg gas" @default.
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• W2045320997 doi "https://doi.org/10.1088/0953-4075/44/18/184019" @default.
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