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• W2045390943 abstract "A model has been developed for the equation of state of deuterium that builds in the correct limiting behavior for the molecular fluid at low pressure and extends smoothly through dissociation to the very high-density monatomic-metallic fluid. The key assumption is that the Helmholtz free energy of the dissociating mixture is a function that can be approximated by the composition average of the free energy of the pure molecular and metallic hydrogen equations of state. The composition is determined by minimizing the free energy. In comparison to earlier studies this model leads to an enhancement of molecular dissociation and a lowering of shock temperatures and pressures. Calculations for shock-compressed liquid deuterium are in agreement with experiments to a pressure of 2.1 Mbar. At about 1 Mbar and 20 000 K liquid deuterium is 90% dissociated and is a nearly degenerate metal. The model predicts that molecular dissociation will lead to negative values of $(ensuremath{partial}P/ensuremath{partial}{T)}_{V}$ in the range 4000 to 10 000 K and volumes below 7 cc/mol. This feature suggests the formation of covalently bonded species in the partially dissociated mixture." @default.
• W2045390943 created "2016-06-24" @default.
• W2045390943 creator A5004660633 @default.
• W2045390943 date "1998-07-01" @default.
• W2045390943 modified "2023-09-27" @default.
• W2045390943 title "Linear-mixing model for shock-compressed liquid deuterium" @default.
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• W2045390943 doi "https://doi.org/10.1103/physrevb.58.669" @default.
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