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- W2045447905 abstract "Calculations are performed to determine the degree of formation of vibrationally excited H+2 by stimulated radiative association. Low energy thermal collisions between the H and H+ are assumed to take place in the presence of an intense radiation field. The parameters in the system include the temperature characterizing the thermal collisions, the width, intensity, and frequency of the stimulating radiation, and the time of flight of the colliding partners in the radiation field. The effect of each parameter on the initial production rate and the radiative equilibrium populations for each vibrational state are discussed. Possible experimental procedures are also considered. The results indicate a rather surprising degree of vibrational selectivity, particularly for the early time populations of the higher states. Relative ’’initial’’ and radiative equilibrium populations and the rate coefficients for stimulated and spontaneous emission and absorption are tabulated for individual vibrational states for a select set of calculations. Absolute populations are not tabulated but can be easily obtained from the data given." @default.
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- W2045447905 date "1979-08-15" @default.
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- W2045447905 title "Formation of vibrationally excited diatomic molecules by stimulated radiative association: Theoretical calculations in H+2" @default.
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- W2045447905 doi "https://doi.org/10.1063/1.438536" @default.
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