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- W2045462281 abstract "Mossbauer studies were performed in 57Fe impurities (0.3% at.) in solid methane, in order to investigate the properties of the order-disorder phase transition taking place at Tc=20.4K. From the temperature dependence of the relative values of the recoil-free-fraction - f - it was found that near Tc a change occurs in the slope of f(T2) without discontinuity in the value of f. A consistent model is proposed by which immediately below Tc both phases, I and II coexist with a gradual evolution of the ordered state (II) on the account of the high temperature plastic state (I). The Debye temperature of phase II (θII = 101±7K) increases with respect to that of phase I (θI = 72±3K), indicating a hardening in the phonon spectrum and precluding the onset of rotational modes of the disordered molecules." @default.
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- W2045462281 date "1978-08-01" @default.
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- W2045462281 title "Probing the phase transition of methane with Mössbauer effect in 57Fe impurities" @default.
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- W2045462281 doi "https://doi.org/10.1016/0038-1098(78)90694-4" @default.
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