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- W2045474505 abstract "It has been shown previously that antimony evaporated onto a Au(111) surface grows in a layer-by-layer mode. The present work compares the initial, fast-oxidation stage of these films with that on bulk polycrystalline antimony. Measurements were carried out in an ultrahigh-vacuum environment using Auger electron spectroscopy, low-energy electron diffraction, electron-energy-loss spectroscopy, and work-function change measurements. At 300 K and for oxygen pressures between 1ifmmodetimeselsetexttimesfi{}${10}^{mathrm{ensuremath{-}}5}$ and 2ifmmodetimeselsetexttimesfi{}${10}^{mathrm{ensuremath{-}}3}$ Torr, oxidation follows first-order Langmuir kinetics, with an initial sticking probability of about ${10}^{mathrm{ensuremath{-}}5}$. Oxidation essentially saturates by ${10}^{7}$ L (1 L=${10}^{mathrm{ensuremath{-}}6}$ Torr s). A layer of oxide about 8.5 AA{} thick is formed in this initial stage, both for Sb films and for bulk antimony. An initial antimony film on Au(111) of about 1.7 monolayers, or 1.6ifmmodetimeselsetexttimesfi{}${10}^{15}$ atoms/${mathrm{cm}}^{2}$, is required to complete this oxide layer, for saturation oxidation. The chemical composition of the oxidized films and the oxidized surface of bulk antimony is ${mathrm{Sb}}_{2}$${mathrm{O}}_{3}$. These results are compared with earlier work on Pb, Bi, and Sn." @default.
- W2045474505 created "2016-06-24" @default.
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- W2045474505 date "1994-03-15" @default.
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- W2045474505 title "Initial oxidation of ultrathin antimony films on Au(111) and of polycrystalline antimony" @default.
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- W2045474505 doi "https://doi.org/10.1103/physrevb.49.8340" @default.
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