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• W2045481166 startingPage "197" @default.
• W2045481166 abstract "The interfacial properties of crystalline zirconium dioxide in aqueous solutions of anionic surfactants at an initial pH value of 3.8 have been studied. Adsorption isotherms, electrophoretic mobilities of the zirconia particles, and the pH of the supernatants were measured for two sodium n-alkyl-p-benzenesulfonates, the heptyl compound (SHBS) and the octyl compound (SOBS), and were compared with those for sodium benzenesulfonate (SBS), a molecule containing no alkyl chain. These traditional experiments were supplemented by calorimetric measurements of the enthalpy of dilution and the enthalpy of adsorption. The system satisfies the condition of charge regulation; the “head-on” adsorption of surfactant ions causes the pH of the equilibrium bulk solution to increase along the isotherm. The patchwise-like topography of the zirconia surface brings about a non-uniform distribution of surface charge and activates tail-tail attraction even at relatively low surface coverages. The primary surface aggregates grow and possibly fuse together in a direction parallel to the surface but for the most part within the surface patches. In consequence, only submonolayer coverages can be achieved, and at higher bulk concentrations aggregates grow into compact and fragmented three-dimensional-like structures." @default.
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• W2045481166 date "1995-05-01" @default.
• W2045481166 modified "2023-09-25" @default.
• W2045481166 title "Interfacial properties of zirconium dioxide in aqueous solutions of sodium alkylbenzenesulfonates" @default.
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• W2045481166 doi "https://doi.org/10.1016/0927-7757(95)03118-w" @default.
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