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• W2045492841 startingPage "17332" @default.
• W2045492841 abstract "Clustering an anion with one or more neutral molecules is a stabilizing process that enhances the oxidation potential of the complex relative to the free ion. Several hydrogen bond clusters (i.e., A(-) • HX, where A(-) = H2PO4(-) and CF3CO2(-) and HX = MeOH, PhOH, and Me2NOH or Et2NOH) are examined by photoelectron spectroscopy and M06-2X and CCSD(T) computations. Remarkably, these species are experimentally found to have adiabatic detachment energies that are smaller than those for the free ion and reductions of 0.47 to 1.87 eV are predicted computationally. Hydrogen atom and proton transfers upon vertical photodetachment are two limiting extremes on the neutral surface in a continuum of mechanistic pathways that account for these results, and the whole gamut of possibilities are predicted to occur." @default.
• W2045492841 created "2016-06-24" @default.
• W2045492841 creator A5041611668 @default.
• W2045492841 creator A5074466299 @default.
• W2045492841 date "2014-12-01" @default.
• W2045492841 modified "2023-09-23" @default.
• W2045492841 title "Anion A^– • HX Clusters with Reduced Electron Binding Energies: Proton vs Hydrogen Atom Relocation upon Electron Detachment" @default.
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• W2045492841 doi "https://doi.org/10.1021/ja510914d" @default.
• W2045492841 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/25409495" @default.
• W2045492841 hasPublicationYear "2014" @default.
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