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• W2045656013 abstract "Abstract Ammonia molecules interact with U atoms, and the resulting U:NH 3 complex rearranges upon visible irradiation to form the H 2 NUH and HNUH 2 molecules in excess argon. These products are identified by functional group frequencies, 15 NH 3 and ND 3 isotopic shifts, and comparison to frequencies calculated by using density functional theory. The NU π bond in HNUH 2 is enhanced by partial triple‐bond character through N(2p) to U(5f) conjugation, which is comparable to that found in the analogous HNThH 2 molecule. These products also form complexes with additional ammonia molecules in the matrix. The interesting higher‐energy NUH 3 complex is not formed." @default.
• W2045656013 created "2016-06-24" @default.
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• W2045656013 date "2008-10-10" @default.
• W2045656013 modified "2023-10-18" @default.
• W2045656013 title "Reactions of Uranium Atoms with Ammonia: Infrared Spectra and Quasi-Relativistic Calculations of the U:NH₃, H₂NUH, and HNUH₂Complexes" @default.
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• W2045656013 doi "https://doi.org/10.1002/chem.200800875" @default.
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