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- W2045673139 abstract "Picosecond time dependent fluorescence depolarization has been used to measure the rotational diffusion time of 3,3′-diethyloxadicarbocyanine iodide (DODCI) in solution at 293 K: the stable form of DODCI was shown to have a “coiled” form, the cis,cis-1,5-conformation, whereas the photoisomer formed by irradiating DODCI in solution was shown to be the elongated all-trans-isomer. The stable form has a rotational correlation time of 160 ± 30 ps in ethanol and 320 ± 40 ps in isopropanol; the fluorescence lifetimes were 1.2 ± 0.1 ns (ethanol) and 1.6 ± 0.1 ns (isopropanol). The all-trans-photoisomer has a rotational correlation of > 700 ps in isopropanol and a fluorescence lifetime of 0.42 ± 0.05 ns. Furthermore, the rotational diffusion times agree closely with those predicted on the basis of the Stokes-Einstein hydrodynamic model, indicating a lack of any solvent attachment to DODCI in solution." @default.
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- W2045673139 date "1977-07-01" @default.
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- W2045673139 title "Rotational diffusion of the mode-locking dye dodci and its photoisomer" @default.
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- W2045673139 doi "https://doi.org/10.1016/0009-2614(77)80430-2" @default.
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